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课题组简介

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本课题组研究方向为天然产物和药物合成、过渡金属催化和不对称催化反应方法学研究。已在Chem. Soc. Rev.、Acc. Chem. Res.、Chem、J. Am. Chem. Soc.、Angew. Chem. Int. Ed.、Nat. Commun.、Adv. Mater.、iScience、Chem. Commun.、Org. Lett.、Chem. Eur. J.、Adv. Synth. Catal.等发表论文90余篇,被包括Science、Nature在内的国际知名刊物引用2800余次,被Nat. Rev. Chem.、Chem. Rev.、Chem. Soc. Rev.、Coord. Chem. Rev.、 Synfacts等进行图文评论或亮点工作介绍50余次,单篇最高引用700余次。

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课题组研究方向

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1.天然产物全合成方向:

近年来合成的天然产物:

2. 有机合成方法学方向:

(1). 碳-氢键活化官能团化及不对称催化反应方法研究

(i). 以在复杂天然产物或药物分子合成中的应用为目标,基于原子和步骤经济理念,设计发展过渡金属催化的C-H键活化官能团化新方法、新试剂、新催化剂。

(ii). 磷中心手性膦酰胺催化的环状1,3-二酮的去对称化对映选择性还原反应。

J. Am. Chem. Soc., 2021, 143, 2994. (Highlight by SYNFACTS 2021, 17, 562)

(iii). 金鸡纳生物碱季铵盐催化的不对称Michael/Aldol串联反应。

Angew. Chem. Int. Ed., 2020, 59, 3834. (Frontispiece Cover)

(2).过渡金属催化的大位阻非活化烯醇衍生物的偶联反应方法研究

开发了一种基于膦酰胺配体的新型环钯催化剂,用于大位阻非活化烯醇类衍生物的高效铃木偶联反应。

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